CasaTunesSync currently requires you install the "full" version of the Microsoft.Net 4.5 framework. If you only have the "client" version installed it will not work.
You can install the "full" framework from:
Click here to download the full version of the Microsoft.Net 4.5 Framework
Download is also available from: http://www.microsoft.com/en-us/download/details.aspx?id=30653
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